Published August 20, 2020 | Version v1
Journal article Open

Strain-induced structural transition in DyBa2Cu3O7−x films grown by atomic layer-by-layer molecular beam epitaxy

Description

We have used atomic layer-by-layer molecular beam epitaxy to synthesize coherently lattice-matched thin films of the high-temperature superconductor DyBa2Cu3O7−x with minimal defect density. A systematic set of x-ray reciprocal-space maps reveals tetragonal and orthorhombic structures with different twinning patterns and elucidates their evolution with the thickness, the oxygenation state, and the epitaxial relationship with the substrate. We also show that films with more pronounced orthorhombicity exhibit lower normal-state resistivities and higher superconducting transition temperatures. These findings provide guidance for the synthesis of optimized superconducting heterostructures and devices.

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Strain-induced structural transition in DyBa2Cu3O7−x films grown by atomic layer-by-layer molecular beam epitaxy.pdf

Additional details

Funding

European Commission
ESTEEM3 – Enabling Science and Technology through European Electron Microscopy 823717