Published March 15, 2020 | Version v1
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Spectroscopic investigations of negatively charged tin-vacancy centres in diamond

  • 1. Fachrichtung Physik, Universität des Saarlandes, Campus E2.6, D-66123 Saarbrücken, Germany
  • 2. Wigner Research Centre for Physics, Institute for Solid State Physics and Optics, Hungarian Academy of Sciences, Hungary
  • 3. Department of Electrical and Electronic Engineering, Tokyo Institute of Technology, Meguro, Tokyo 152-8552, Japan
  • 4. Advanced Materials Laboratory, National Institute for Material Science, 1-1 Namiki, Tsukuba, 305-0044, Japan
  • 5. Division of Applied Quantum System, Felix Bloch Institute for Solid State Physics, University of Leipzig, D-04103, Leipzig

Description

Spectroscopic investigations of negatively charged tin-vacancy centres in diamond
The recently discovered negatively charged tin-vacancy centre in diamond is a promising candidate for applications in quantum information processing (QIP). We here present a detailed spectroscopic study encompassing single photon emission and polarisation properties, the temperature dependence of emission spectra as well as a detailed analysis of the phonon sideband and Debye–Waller factor. Using photoluminescence excitation spectroscopy we probe an energetically higher lying excited state and prove fully lifetime limited linewidths of single emitters at cryogenic temperatures. For these emitters we also investigate the stability of the charge state under resonant excitation. These results provide a detailed insight into the spectroscopic properties of the SnV− centre and lay the foundation for further studies regarding its suitability in QIP.

Notes

This work was supported by the Joint Research Project SIQUST (17FUN06). This project received funding from the European Metrology Programme for Innovation and Research (EMPIR) cofinanced by the Participating States and from the European Unions Horizon 2020 research and innovation programme.

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Related works

Is supplement to
Journal article: 10.1088/1367-2630/ab6631 (DOI)