Published November 4, 2022 | Version v3
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Unravelling the Nature of the Spin Excitations Disentangled from the Charge Contributions in a Doped Cuprate Superconductor

  • 1. Photon Science Division, Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen PSI, Switzerland
  • 2. Institute of Theoretical Physics, Faculty of Physics, University of Warsaw, Pasteura 5, PL-02093 Warsaw, Poland
  • 3. Department of Quantum Matter Physics, University of Geneva, Quai Ernest-Ansermet 24, CH-1211 Genève 4, Switzerland
  • 4. Institute for Theoretical Solid State Physics, IFW Dresden, 01171 Dresden, Germany

Description

The nature of the spin excitations in superconducting cuprates is a key question toward a unified understanding of the cuprate physics from long-range antiferromagnetism to superconductivity. The intense spin excitations up to the over-doped regime revealed by resonant inelastic X-ray scattering bring new insights as well as problems—like understanding their persistence or their relation to the collective excitations in ordered magnets (magnons). Here, we study the evolution of the spin excitations upon hole-doping the superconducting cuprate Bi2Sr2CaCu2O8+δ by disentangling the spin from the charge excitations in the experimental cross section. We compare our experimental results against density matrix renormalization group calculations for a t-J-like model on a square lattice. Our results unambiguously confirm the persistence of the spin excitations, which are closely connected to the persistence of short-range magnetic correlations up to high doping. This suggests that the spin excitations in hole-doped cuprates are related to magnons—albeit short-ranged.

Notes

The experiments were performed at the ADRESS beamline of the Swiss Light Source at the Paul Scherrer Institut (PSI). The experimental work at PSI is supported by the Swiss National Science Foundation through project no. 200021_178867, and the Sinergia network Mott Physics Beyond the Heisenberg Model (MPBH) (SNSF Research Grants CRSII2 160765/1 and CRSII2 141962). The theoretical work is supported by the Narodowe Centrum Nauki (NCN, Poland) under Project Nos. 2016/22/E/ST3/00560 (C.E.A. and K.W.), 2021/40/C/ST3/00177 (C.E.A.) and 2016/23/B/ST3/00839 (K.W.). We acknowledge sup- port by the Interdisciplinary Centre for Mathematical and Computational Modeling (ICM), University of Warsaw (UW), within grant no G81-4. S.N. acknowledges support from SFB 1143 project A05 (project-id 247310070) of the Deutsche Forschungsgemeinschaft. T.C.A. acknowledges funding from the European Union's Horizon 2020 research and innovation programme under the Marie Sklodowska-Curie grant agreement No. 701647 (PSI-FELLOW-II-3i program).

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UnravellingNatureofSpinAndChargeExcitations-theory+expData.zip

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Related works

Is referenced by
Preprint: 10.48550/arXiv.2204.08749 (DOI)

Funding

Mott Physics Beyond the Heisenberg Model in Iridates and Related Materials CRSII2_160765
Swiss National Science Foundation
Electron-Phonon Interactions in Rare-Earth Nickelates and Superconducting Cuprates 200021_178867
Swiss National Science Foundation
Mott Physics Beyond the Heisenberg Model in Iridates and Related Materials CRSII2_141962
Swiss National Science Foundation