Published April 10, 2020 | Version v1
Dataset Open

Dataset for "InGaN Nanohole Arrays Coated by Lead Halide Perovskite Nanocrystals for Solid-State Lighting"

  • 1. Experimental Condensed Matter Physics Laboratory, Department of Physics, University of Cyprus, Nicosia 1678, Cyprus
  • 2. Institute of Inorganic Chemistry, Department of Chemistry and Applied Biosciences, ETH Zürich, CH-8093 Zürich, Switzerland; Laboratory for Thin Films and Photovoltaics, Empa−Swiss Federal Laboratories for Materials Science and Technology, CH-8600 Dübendorf, Switzerland
  • 3. Department of Electronic and Electrical Engineering, University of Sheffield, Sheffield S1 4DE, United Kingdom
  • 4. Department of Electronic and Electrical Engineering, University of Bath, Bath BA2 7AY, United Kingdom
  • 5. Institute of Inorganic Chemistry, Department of Chemistry and Applied Biosciences, ETH Zürich, CH-8093 Zürich, Switzerland

Description

In this work, we demonstrate efficient light downconversion via FRET in InGaN/GaN multiple quantum well (MQW) nanohole arrays, coated with green-emitting CsPbBr3 and FAPbBr3 nanocrystals (NCs) and near-infrared (IR) FAPbI3 NC overlayers for solid-state lighting. Patterning the InGaN MQW into nanohole arrays allows a minimum nitride−NC separation while increasing the heterointerfacial area, thus improving simultaneously the nonradiative and radiative transfer efficiencies. Detailed spectroscopic studies of steady-state and time-resolved photoluminescence indicate a significant reduction in the quantum well photoluminescent decay time in the presence of NCs, accompanied by a significant concurrent increase of the NC integrated emission, providing evidence of efficient light down-conversion mediated by FRET with efficiencies as high as ∼83 ± 6% in the green and ∼74 ± 5% in the near-IR.

Files

Figure 1(d) CsPbBr3 TEM.jpg

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Additional details

Funding

PEROGAN – Novel Light Emitters based on Nanostructures of III-Nitrides and Lead Halide Perovskite Nanocrystals 831690
European Commission