Published March 28, 2022 | Version v1
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Entropy driven order in an array of nanomagnets

  • 1. Yale University
  • 2. Los Alamos National Laboratory
  • 3. University of Illinois Urbana-Champaign
  • 4. Wayne State University
  • 5. University of Minnesota
  • 6. University of Liverpool
  • 7. Lawrence Berkeley National Laboratory

Description

Long-range ordering, while typically understood as a decrease in entropy, can also be driven by increasing system entropy in certain special cases. We demonstrate that artificial spin ice arrays of single-domain nanomagnets can be designed to produce entropy-driven order. We probe thermally active tetris artificial spin ice, known to have a zero point Pauli entropy, both experimentally and through simulations. We find two-dimensional magnetic ordering in one subset of the nanomagnet moments, which we demonstrate to be induced by disorder (i.e., increased entropy) in another subset of moments. Contrasting with other entropy-driven systems, the degrees of freedom in artificial spin ice are both designable and directly observable at the microscale, and the entropy of the system is precisely calculable in simulations. This robust example, in which the system's interactions and ground state entropy are well-defined, significantly expands the experimental landscape for the study of entropy-driven ordering.

Notes

Funding provided by: U.S. Department of Energy
Crossref Funder Registry ID: http://dx.doi.org/10.13039/100000015
Award Number: DE-SC0010778

Funding provided by: U.S. Department of Energy
Crossref Funder Registry ID: http://dx.doi.org/10.13039/100000015
Award Number: DE-SC0020162

Funding provided by: U.S. Department of Energy
Crossref Funder Registry ID: http://dx.doi.org/10.13039/100000015
Award Number: DE-AC02-05CH11231

Funding provided by: National Science Foundation
Crossref Funder Registry ID: http://dx.doi.org/10.13039/100000001
Award Number: DMR-1807124

Funding provided by: National Science Foundation
Crossref Funder Registry ID: http://dx.doi.org/10.13039/100000001
Award Number: DMR-2103711

Funding provided by: UK Royal Society*
Crossref Funder Registry ID:
Award Number: RGS\R2\180208

Funding provided by: Triad National Security*
Crossref Funder Registry ID:
Award Number: 892333218NCA000001

Funding provided by: U.S. Department of Energy - LDRD*
Crossref Funder Registry ID:
Award Number:

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Related works

Is source of
10.5061/dryad.rbnzs7hcs (DOI)