Published 2025 | Version v2
Dataset Open

Observation of a hidden charge density wave liquid

Authors/Creators

  • 1. ROR icon University of California, Los Angeles

Contributors

Supervisor:

  • 1. ROR icon University of California, Los Angeles

Description

Charge density waves (CDWs), electronic crystals that form within a host solid, have long been theorized to melt into a spatially textured electronic liquid. Although such liquid CDWs have not been previously observed, they may be central to the phase diagrams of correlated electron systems, including high-temperature superconductors and quantum Hall states. In 1T-TaS2, a promising material for hosting a liquid CDW, a structural phase transition hinders observation. Here, we use femtosecond light pulses to bypass this transition, revealing how topological defect dynamics govern hidden CDW correlations. Following photoexcitation, CDW diffraction peaks broaden azimuthally, indicating the emergence of a hexatic state. At elevated temperatures, photoexcitation fully destroys both translational and orientational order, leaving only a ring of diffuse scattering—a hallmark of a liquid CDW. These findings offer compelling evidence for a defect-unbinding transition into a CDW liquid. More broadly, this approach demonstrates a route to uncover electronic phases obscured by intervening transitions in thermal equilibrium.

Files

360K_differential_averaged_data.zip

Files (4.7 GB)

Name Size Download all
md5:276533e068576d98afa3e456ba00d330
14.8 MB Preview Download
md5:ee275ddf95c415d65fab7fe6735e6d57
523.9 MB Preview Download
md5:71adeaffb3b1221da3b1d01942699e38
488.7 MB Preview Download
md5:66c83eaedccfc3240c2b33066c30fcd2
540.8 MB Preview Download
md5:ffc1eba23f0343e2a2574640b9dc4888
493.2 MB Preview Download
md5:97e609305f19cfe1f5dd80eae2779a14
528.8 MB Preview Download
md5:314f8436dca74637e974f2d524f7db5d
505.1 MB Preview Download
md5:42dfd71c97bc6a8e29706993999ffd01
18.1 MB Preview Download
md5:312d4a8339900d205e4faae2162591b6
624.1 MB Preview Download
md5:9afd5a65e8a30f61d318ad6c346a0265
640.6 MB Preview Download
md5:e76c9ace56ea9ca917210c8d9b7e3e11
145.5 MB Preview Download
md5:bb376cb74b095de2f25e6f6dbe598d84
5.5 MB Preview Download
md5:0a5a5f86b67495cf0c53f368f97257d5
4.2 MB Preview Download
md5:3ef1422e6480d5762e0356ded454214e
25.2 kB Preview Download
md5:749e029a9fcfebcb4f8773d1ed1d99d5
170 Bytes Preview Download
md5:54aca316c70baf5de1aab913cd5f195b
25.2 MB Preview Download
md5:d5d77f06f442cf5393ea843fb168f26f
1.4 kB Preview Download
md5:b8af3d9efd21db20926df08f3bc60321
902 Bytes Preview Download
md5:fa588ba471b8cf1fa522002b1f35ffe7
2.8 kB Preview Download
md5:408fe7f2459c309e836bbff8192a9e3c
892 Bytes Preview Download
md5:86e5cfb1a3bcbf79d5589de663d0e50c
643.4 kB Preview Download
md5:519ba0928b38055ef8ed0a7f88873ff3
41.7 kB Preview Download
md5:6b15cf9fd5f1ea63bf3f5fd8f24fcaba
643.4 kB Preview Download
md5:f25c9597736638077a10c4e57943708a
643.4 kB Preview Download
md5:755ec6c76d40eba7b11eb3dee7dacc8c
643.4 kB Preview Download
md5:56c6303f10ee8b584471c97c9b59f547
25.2 MB Preview Download
md5:99b404a5a1b40d3c4dc4767ca6b127c5
1.6 kB Preview Download
md5:75b6756dea9210a2310d8b21d4fa5c4f
1.1 kB Preview Download
md5:812b07a8645f052e38bc2d4c602ae49e
2.8 kB Preview Download
md5:c05cb74b2815df89227394daeccde127
1.1 kB Preview Download
md5:8685ab6521270847d5e05eb4a6a5d38c
653.1 kB Preview Download
md5:fb59bf00fefee1944dc9a3f9d2666b5a
42.2 kB Preview Download
md5:05718be9f7499794d63ec041a362b7b3
654.7 kB Preview Download
md5:89407cdd422de9861a72ddb193568e18
654.7 kB Preview Download
md5:b268bbe6183b9157e63e2d715f98b5a9
654.7 kB Preview Download
md5:755ec6c76d40eba7b11eb3dee7dacc8c
643.4 kB Preview Download
md5:2065c547126c96f2a05398e7b8a5b96a
641.8 kB Preview Download
md5:188ec8ef1f2deea709a670b83e1f698e
641.8 kB Preview Download
md5:8b3593d08ffc8b3b2ddc592d327b514b
641.8 kB Preview Download
md5:79bc1fd9fa2461a5940a0329be8c9e0c
641.8 kB Preview Download
md5:64a6814bcba5080dd9eeb2f96cb9d497
654.7 kB Preview Download
md5:80dadf8de2d324d8214b15f91e2c53f9
97.9 kB Preview Download
md5:2dfda852c3cd1784c052aa3247e53561
164 Bytes Preview Download
md5:b6df6a850b21d93f5228f58efe0ff872
166 Bytes Preview Download
md5:c170ddd5c91564e511b2aa1f999fc3e6
171 Bytes Preview Download
md5:df3723d3defa75b934b4b8b7a4f65f3d
2.0 MB Preview Download
md5:290b3e3c04a0e7d984a3c85efb1ba3a0
47.3 MB Preview Download
md5:a08404835d0b7fae2063088870279c6b
64.6 MB Preview Download
md5:14fd758236e3b9842cbb8ea46ff4d723
3.6 kB Preview Download
md5:5a4ff5484b1a72dfe2432b8b2842c97f
4.5 kB Preview Download
md5:1d5cdec37c7b118a849b7964cb00ce62
648.3 kB Preview Download
md5:fd705dd0e6a5b63a5a52c70a08570997
648.2 kB Preview Download
md5:cd2263739a8eb5d78028a47ad775f55d
648.2 kB Preview Download
md5:8c9c24d6731fbe5b337c2027fed87388
648.2 kB Preview Download
md5:b86b306b020eab97fa7d90791dd8fc07
15.0 kB Preview Download
md5:7c750f90f54a711fb6bd0b52829217fb
7.0 kB Preview Download
md5:b3d761baf11d32e03aa4b11c02c112d8
1.5 kB Preview Download
md5:b60afb37cdc6ac461218aee3a03c540d
1.5 kB Preview Download
md5:f9eced1bd3d49b20307a49283cf590c3
6.5 kB Preview Download
md5:aa27782b050cd1aa4880988aff0e867c
2.5 kB Preview Download
md5:f190fe8429ad5f9a84bc069e637e3c1e
1.7 kB Preview Download
md5:ec579d29a6d89294a30d87611a5012f6
1.9 kB Preview Download
md5:873db9a6eb153d913a7662e4a43fe8ac
19.5 kB Preview Download
md5:0a75709ea232a3344a5eec998c9172fc
136 Bytes Preview Download
md5:bc475cd823b38f5213192715adac23dd
625.9 kB Preview Download
md5:1fac2db6aae475f066bc2331ee863ef5
624.3 kB Preview Download
md5:66f83e52ecfe8caab1cae1f587fdcbd0
624.3 kB Preview Download
md5:4a96178f90c4188d18971e458c4c5ae8
624.3 kB Preview Download
md5:ed45eb15640757cf321300bd0dbd3e2c
39.9 kB Preview Download
md5:458b1dbf1c68f43ebaf87a514cf1ca5e
472 Bytes Preview Download
md5:b8869c29278e20ccde42e1283b56d7d6
536 Bytes Preview Download