Published August 18, 2025
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Vibronic coupling limits the use of high-lying electronic states in complex molecules for laser cooling
Authors/Creators
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1.
University of California, Los Angeles
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2.
University of Southern California
Description
The data set composes all spectra shown in the paper "Vibronic coupling limits the use of high-lying electronic states in complex molecules
for laser cooling". The paper aims to explore the optical cycling properties of the third electronic excited state C for CaOPh and SrOPh molecules. We find that non-
adiabatic couplings between the A, B, and C states lead to substantial mixing, giving rise to vibronic states that enable additional decay pathways. As such, vibronic couplings limits the use of higher electronic states for laser cooling purposes.
Files
All Spectra.zip
Files
(389.2 kB)
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