Published September 15, 2015 | Version v1
Journal article Open

The effect of Gd on trityl-based dynamic nuclear polarisation in solids

  • 1. Magnetic Resonance Center (CERM) and Department of Chemistry "Ugo Schiff", University of Florence, Italy
  • 2. Chemical Physics Department, Weizmann Institute of Science, Rehovot, Israel
  • 3. Fondazione CNR/Regione Toscana G. Monasterio and Institute of Life Sciences, Scuola Superiore Sant'Anna, Pisa, Italy
  • 4. Fondazione CNR/Regione Toscana G. Monasterio and Institute of Clinical Physiology, National Council of Research, Pisa, Italy

Description

The increase in 13C polarisation of 13C-urea dissolved in samples containing water/DMSO mixtures and trityl radical (OX063) in the presence of Gd3+ is explained by changes in electron relaxation, electron spectral diffusion and effective electron–proton hyperfine interaction.

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Funding

European Commission
PNMR - Pushing the Envelope of Nuclear Magnetic Resonance Spectroscopy for Paramagnetic Systems. A Combined Experimental and Theoretical Approach 317127