Raw 1H NMR and photo-CIDNP-enhanced NMR data. This data is described in the associated publication "Optically Enhanced Solid-State 1H NMR Spectroscopy" www.doi.org/10.1021/jacs.3c03937 NMR data is given in the form of raw free induction decay (FID) files, where the first column is time (in microseconds), and second and third columns are the quadrature-detected FID data (arbitrary units). Data are organized in folders, each corresponding to the associated figure in the manuscript and in the supporting information. Further information are given in the "fig_XX_exp_cond.txt" files and in each figure caption. Data are processed with a Mathematica notebook included here in the "processing" folder. For the processing, the first 22 points of the FIDs are removed so that the half-echo and not the full-echo is Fourier-transformed to obtain the spectrum. Only 1800 points in the FID are considered. Typically, a line broadening of 5 kHz is applied to improve the signal-to-noise ratio. For the laser-on experiments, the following equivalences between laser power and intensity hold true: 1) 0.07 W <--> 1.0 W cm^-2 2) 0.17 W <--> 2.4 W cm^-2 3) 0.27 W <--> 3.8 W cm^-2 4) 0.37 W <--> 5.2 W cm^-2 5) 0.47 W <--> 6.6 W cm^-2