Published July 11, 2022 | Version v1
Journal article Open

Magneto-Ionics in Annealed W/CoFeB/HfO2 Thin Films

  • 1. Centre de Nanosciences et de Nanotechnologies CNRS Université Paris-Saclay Palaiseau 91120, France
  • 2. Laboratoire des Sciences des Procédés et des Matériaux CNRS-UPR 3407 Université Sorbonne Paris Nord Villetaneuse 93430, France
  • 3. Singulus Technology AG Hanauer Landstrasse 103 63796, Kahl am Main, Germany
  • 4. IMM-CNR Unit of Agrate Brianza Via C. Olivetti 2, Agrate Brianza 20864, Italy
  • 5. Spin-Ion Technologies 10 Boulevard Thomas Gobert, Palaiseau 91120, France
  • 6. Istituto Nazionale di Ricerca Metrologica Strada delle Cacce 91, Torino 10135, Italy and Politecnico di Torino Viale duca degli Abruzzi 24, Torino 10129, Italy
  • 7. Univ. Grenoble Alpes, CNRS, Institut Néel Grenoble 38000, France
  • 8. Center for Superconductivity Spintronics and Surface Science Physics and Chemistry Department Technical University of Cluj-Napoca Cluj-Napoca RO-400114, Romania
  • 9. Istituto Nazionale di Ricerca Metrologica Strada delle Cacce 91, Torino 10135, Italy
  • 10. Central Research Institute of Electric Power Industry Yokosuka, Kanagawa 240-0196, Japan

Description

 The magneto-ionic modulation of the Dzyaloshinskii–Moriya interaction

(DMI) and the perpendicular magnetic anisotropy (PMA), in W/CoFeB/HfO2

 stacks annealed at different temperatures and for varying annealing times,

are presented in this work. A large modulation of PMA and DMI is observed

in the systems annealed at 390 and 350 ° C, whereas no response to voltage is

observed in the as-grown samples. A strong DMI is only observed in the samples

annealed at 390 ° C for 1 h, while PMA is present for all annealing times

at temperatures of 390 and 350 ° C. Magnetic properties including domain

wall velocity improve drastically with increasing the annealing temperature

and time, while the magneto-ionic reversibility is increasingly compromised.

The changes in PMA and DMI induced by the gate voltages in the samples

annealed at 390 ° C are permanent, while partial reversibility is only observed

for the samples annealed at 350 ° C for short times. This dependence of reversibility

on post-grown annealing has been associated to the influence of crystallization

on ion mobility. These results show that a compromise between the

enhancement of the magnetic properties and the magneto-ionic performance

could be needed in systems requiring annealing to develop PMA and DMI.

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Additional details

Funding

MagnEFi – Magnetism and the effects of Electric Field 860060
European Commission