DOI: 10.5281/zenodo.16600544 URL: https://doi.org/10.5281/zenodo.16600544 This raw data repository supports the publication 'Low-Temperature Depolymerization of Polymethacrylamides' published in Angewandte Chemie International Edition 2025, 64, 22, e202425575 https://doi.org/10.1002/anie.202425575 it includes all the raw data plotted in the figures of the manuscript. The collection inlcudes the file 'experimental_overview.csv'. All experiments are named according to the following nomenclature: 'VL-Exp.No-Sample No' The experimental conditions behind the experiment numbers are summarized in the overview file in addition to the figure number they belong to. SEC raw data includes to tables for each sample with one corresponding to the refractive index signal (Detector B) and one to the UV signal (Detector A) against the retention time. NMR data is the raw data compiled in a zip file for each sample, which can be opened with any NMR analysis software (e.g. MestreNova, Topshim). Statistical analysis was conducted with the included R script and data set in file 'Fig4_statisticalanalysis.zip'.