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We discuss the peculiarities of the Seebeck effect in stabilized electrolytes containing the colloidal particles. Its unusual feature is the two stage character, with the linear increase of differential thermopower as the function of colloidal particles concentration n\u2299 during the first stage (“initial state”) and dramatic drop of it at small n\u2299 during the second one (“steady state”). We show that the properties of the initial state are governed by the thermo-diffusion flows of the mobile ions of the stabilizing electrolyte medium itself and how the colloidal particles participate in the formation of the electric field in the bulk of the suspension. In its turn, we attribute the specifics of the steady state thermoelectric effect the massive colloidal particles undergoing slow thermal diffusion and the break down of their electro-neutrality in the vicinity of electrodes
", "publication_date": "2021-01-26", "publisher": "Zenodo", "resource_type": { "id": "publication-article", "title": { "de": "Zeitschriftenartikel", "en": "Journal article" } }, "rights": [ { "description": { "en": "The Creative Commons Attribution license allows re-distribution and re-use of a licensed work on the condition that the creator is appropriately credited." }, "icon": "cc-by-icon", "id": "cc-by-4.0", "props": { "scheme": "spdx", "url": "https://creativecommons.org/licenses/by/4.0/legalcode" }, "title": { "en": "Creative Commons Attribution 4.0 International" } } ], "title": "Two-Stage Seebeck Effect in Charged Colloidal Suspensions" }, "parent": { "access": { "owned_by": { "user": 33303 } }, "communities": { "default": "07accaa2-92d3-482b-aa99-59f7993a0bf8", "entries": [ { "access": { "member_policy": "open", "members_visibility": "public", "record_policy": "open", "review_policy": "open", "visibility": "public" }, "children": { "allow": false }, "created": "2017-07-19T20:00:07.512474+00:00", "custom_fields": {}, "deletion_status": { "is_deleted": false, "status": "P" }, "id": "07accaa2-92d3-482b-aa99-59f7993a0bf8", "links": {}, "metadata": { "curation_policy": "", "page": "In the MAGENTA H2020 project we are developing brand new thermoelectric materials based on ionic ferrofluids; i.e., colloidal dispersions of magnetic nanoparticles in ionic liquids. It is an inter-disciplinary and cross-sector R&D project combining concepts and techniques from physics, chemistry and electrochemistry with an active participation from industrial partners. As its final products, MAGENTA will offer novel liquid thermoelectric materials that are versatile, cost-effective and non-toxic to assist the economically and environmentally sustainable energy transition in Europe.
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