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Small-angle neutron scattering and magnetically heterogeneous state in Sr2FeMoO6–δ

Nikolay Kalanda; Vasil Garamus; Mikhail Zheludkevich; Marta Yarmolich; Maria Serdechnova; Dietmar Christian Florian Wieland; Alexander Petrov; Aliaksandr Zhaludkevich; Nikolai A. Sobolev


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  <identifier identifierType="DOI">10.5281/zenodo.3691820</identifier>
  <creators>
    <creator>
      <creatorName>Nikolay Kalanda</creatorName>
      <affiliation>Scientific-Practical Materials Research Centre of the NAS of Belarus, P. Brovka str. 19, 220072 Minsk, Belarus</affiliation>
    </creator>
    <creator>
      <creatorName>Vasil Garamus</creatorName>
      <affiliation>Helmholtz–Zentrum Geesthacht: Zentrum für Material- und Küstenforschung GmbH, Max–Planck–Str. 1, D–21502 Geesthacht, Germany</affiliation>
    </creator>
    <creator>
      <creatorName>Mikhail Zheludkevich</creatorName>
      <affiliation>Helmholtz–Zentrum Geesthacht: Zentrum für Material- und Küstenforschung GmbH, Max–Planck–Str. 1, D–21502 Geesthacht, Germany</affiliation>
    </creator>
    <creator>
      <creatorName>Marta Yarmolich</creatorName>
      <affiliation>Scientific-Practical Materials Research Centre of the NAS of Belarus, P. Brovka str. 19, 220072 Minsk, Belarus</affiliation>
    </creator>
    <creator>
      <creatorName>Maria Serdechnova</creatorName>
      <affiliation>Helmholtz–Zentrum Geesthacht: Zentrum für Material- und Küstenforschung GmbH, Max–Planck–Str. 1, D–21502 Geesthacht, Germany</affiliation>
    </creator>
    <creator>
      <creatorName>Dietmar Christian Florian Wieland</creatorName>
      <affiliation>Helmholtz–Zentrum Geesthacht: Zentrum für Material- und Küstenforschung GmbH, Max–Planck–Str. 1, D–21502 Geesthacht, Germany</affiliation>
    </creator>
    <creator>
      <creatorName>Alexander Petrov</creatorName>
      <affiliation>Scientific-Practical Materials Research Centre of the NAS of Belarus, P. Brovka str. 19, 220072 Minsk, Belarus</affiliation>
    </creator>
    <creator>
      <creatorName>Aliaksandr Zhaludkevich</creatorName>
      <affiliation>Scientific-Practical Materials Research Centre of the NAS of Belarus, P. Brovka str. 19, 220072 Minsk, Belarus</affiliation>
    </creator>
    <creator>
      <creatorName>Nikolai A. Sobolev</creatorName>
      <affiliation>Departamento de Física and I3N, Universidade de Aveiro, 3810–193 Aveiro, Portugal &amp; National University of Science and Technology MISiS, 119049 Moscow, Russia</affiliation>
    </creator>
  </creators>
  <titles>
    <title>Small-angle neutron scattering and magnetically heterogeneous state in Sr2FeMoO6–δ</title>
  </titles>
  <publisher>Zenodo</publisher>
  <publicationYear>2019</publicationYear>
  <subjects>
    <subject>strontium ferromolybdate</subject>
    <subject>superstructure ordering</subject>
    <subject>oxygen non-stoichiometry</subject>
    <subject>magnetization</subject>
    <subject>small-angle neutron scattering</subject>
  </subjects>
  <dates>
    <date dateType="Issued">2019-05-09</date>
  </dates>
  <language>en</language>
  <resourceType resourceTypeGeneral="JournalArticle"/>
  <alternateIdentifiers>
    <alternateIdentifier alternateIdentifierType="url">https://zenodo.org/record/3691820</alternateIdentifier>
  </alternateIdentifiers>
  <relatedIdentifiers>
    <relatedIdentifier relatedIdentifierType="DOI" relationType="IsPreviousVersionOf" resourceTypeGeneral="JournalArticle">10.1002/pssb.201800428</relatedIdentifier>
    <relatedIdentifier relatedIdentifierType="DOI" relationType="IsVersionOf">10.5281/zenodo.3691819</relatedIdentifier>
  </relatedIdentifiers>
  <version>Author Accepted Manuscript</version>
  <rightsList>
    <rights rightsURI="https://creativecommons.org/licenses/by/4.0/legalcode">Creative Commons Attribution 4.0 International</rights>
    <rights rightsURI="info:eu-repo/semantics/openAccess">Open Access</rights>
  </rightsList>
  <descriptions>
    <description descriptionType="Abstract">&lt;p&gt;Single-phase strontium ferromolybdate (Sr2FeMoO6&amp;ndash;&amp;delta;) samples with different degrees of the superstructural ordering of the Fe/Mo cations were obtained from partially reduced SrFeO3&amp;ndash;х, SrMoO4 precursors by the solid-state technology. The study of the temperature dependences of the magnetization measured in the field-cooling and zero-field-cooling regimes indicated an inhomogeneous magnetic state of the samples. The presence of magnetic regions of different nature has also been revealed by the small-angle neutron scattering. For the Sr2FeMoO6&amp;ndash;&amp;delta; samples with different superstructural ordering of the Fe/Mo cations and for all values of the magnetic field induction in the range up to 1.5 T and of the scattering vector in the interval 0.1 &amp;gt;q &amp;gt;0.005 &amp;Aring;&amp;ndash;1, the analytical dependence I ~ q&amp;ndash;&amp;alpha; obeys the Porod law (&amp;alpha; &amp;asymp; 4), which corresponds to an object with a smooth and well-marked surface and polydisperse grain size. Deviations from the Porod law in the q &amp;gt; 0.1 &amp;Aring;&amp;ndash;1 region and a weakening of the neutron scattering in applied magnetic fields may be ascribed to magnetic inhomogeneities with diameters D &amp;lt;6 nm, which are partially destroyed /oriented by magnetic fields В &amp;ge;1.5 T.&amp;nbsp;&lt;/p&gt;</description>
  </descriptions>
  <fundingReferences>
    <fundingReference>
      <funderName>European Commission</funderName>
      <funderIdentifier funderIdentifierType="Crossref Funder ID">10.13039/100010661</funderIdentifier>
      <awardNumber awardURI="info:eu-repo/grantAgreement/EC/H2020/778308/">778308</awardNumber>
      <awardTitle>Physical principles of the creation of novel SPINtronic materials on the
base of MULTIlayered metal-oxide FILMs for magnetic sensors and MRAM</awardTitle>
    </fundingReference>
  </fundingReferences>
</resource>
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