Journal article Open Access

Vaporization behaviour of the Molten Salt Fast Reactor fuel: The LiF-ThF4-UF4 system

Tosolin, A.; O. Beneš; J.-Y. Colle; P. Soucek; L. Luzzi; R.J.M. Konings


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    <subfield code="a">Knudsen effusion mass spectrometry</subfield>
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    <subfield code="a">Vapour pressure</subfield>
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    <subfield code="a">Vaporization behaviour of the Molten Salt Fast Reactor fuel: The LiF-ThF4-UF4 system</subfield>
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    <subfield code="c">661891</subfield>
    <subfield code="a">A Paradigm Shift in Reactor Safety with the Molten Salt Fast Reactor</subfield>
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    <subfield code="a">&lt;p&gt;A selected composition of the initial fuel of the Molten Salt Fast Reactor (MSFR) is assessed by differential&lt;/p&gt;

&lt;p&gt;scanning calorimetry (DSC) for melting point determination and by Knudsen effusion mass spectrometry&lt;/p&gt;

&lt;p&gt;(KEMS) for vaporization behaviour. Partial vapour pressures and thermodynamic activities of the MSFR&lt;/p&gt;

&lt;p&gt;fuel mixture are discussed indicating departures from ideal behaviour, and further interpreted by phase&lt;/p&gt;

&lt;p&gt;equilibria calculations. The boiling point of the mixture is obtained extrapolating vapour pressure&lt;/p&gt;

&lt;p&gt;experimental results. New results on the vaporization behaviour of pure uranium tetrafluoride are&lt;/p&gt;

&lt;p&gt;presented, together with the ionization potentials of UF4 by electron impact.&lt;/p&gt;</subfield>
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